EGU21-13554
https://doi.org/10.5194/egusphere-egu21-13554
EGU General Assembly 2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.

NOx emissions from U.S. oil and gas production using TROPOMI NO2 and the divergence method

Barbara Dix1, Colby Francoeur1,2, Brian McDonald2, Raquel Serrano3, Pepijn Veefkind3,4, Pieternel Levelt3,4, and Joost de Gouw1,5
Barbara Dix et al.
  • 1University of Colorado, CIRES, Boulder, USA (barbara.dix@colorado.edu)
  • 2NOAA Chemical Sciences Laboratory, Boulder, CO, USA
  • 3Technical University of Delft, Department of Geoscience and Remote Sensing , Delft, the Netherlands
  • 4Royal Netherlands Meteorological Institute (KNMI), De Bilt, the Netherlands
  • 5University of Colorado, Department of Chemistry, Boulder, CO, USA

The development of horizontal drilling and hydraulic fracturing has led to a steep increase in the U.S. production of natural gas and crude oil from shale formations since the mid 2000s. Associated with this industrial activity are emissions of ground-level ozone precursors such as nitrogen oxides (NOx). Satellite data are important in this context, because surface measurements are limited or non-existent in rural regions, where most U.S. oil and gas production operations take place. Here we use TROPOMI NO2 observations to study NOx emissions coming from oil and natural gas production sites. Applying the divergence method we quantify basin wide emissions from well pad fields and aim to push spatial and temporal resolution of this technique. The divergence was method introduced by Beirle et al. (Science Advances 2019) to quantify point source emissions. It relies on calculating the divergence of the NO2 flux to derive NOx sources and estimating the NO2 lifetime to quantify sinks. Our analysis will include an assessment of different methods to constrain the NO2 lifetime, which becomes particularly important when applying this method to larger areas. Further we will compare our results with bottom-up derived emissions. Here we use the Fuel-based Oil & Gas (FOG) inventory that calculates NOx emissions based on fuel consumption. Initial results show good agreement for the Permian Basin (NM, TX) and we will expand our analysis to other U.S. basins.

How to cite: Dix, B., Francoeur, C., McDonald, B., Serrano, R., Veefkind, P., Levelt, P., and de Gouw, J.: NOx emissions from U.S. oil and gas production using TROPOMI NO2 and the divergence method, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13554, https://doi.org/10.5194/egusphere-egu21-13554, 2021.

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