EGU21-3744
https://doi.org/10.5194/egusphere-egu21-3744
EGU General Assembly 2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.

Americium-241 in peat bogs as a marker of the beginning of the Anthropocene: examples from Europe and North America.

Andrii Oleksandrenko1, Peter Appleby2, Tommy Noernberg1, and William Shotyk1
Andrii Oleksandrenko et al.
  • 1Department of Renewable Resources, University of Alberta, Edmonton, Alberta, Canada
  • 2Department of Mathematical Sciences, University of Liverpool, Liverpool, UK

Americium-241 (241Am) is present in the terrestrial and aquatic environment around the globe as a result of the atmospheric testing of high yield thermonuclear weapons carried out mainly in the 1950s and 1960s. Radioactive debris (including mainly 137Cs, 90Sr, and various Pu isotopes) from the tests was injected high into the stratosphere where it was rapidly dispersed around the world. Over a period of months this material slowly returned to the troposphere, and from there was quickly removed by wet and dry fallout onto the earth’s surface. Amounts of 241Am in freshly deposited weapons test debris were essentially zero. Its presence today is through in-growth from its short-lived precursor 241Pu (half-life 14.4 years). By this process concentrations of 241Am have steadily increased with time and will continue to do so through to around 2040. Widely considered to be immobile in soils and sediments, with its well-known origins and long half-life (432 years), 241Am is in many ways an ideal chronostratigraphic marker of the nuclear age. Calculations show that the 241Am record in any ideal natural archive is a faithful representation of the history of weapons test fallout. Beginning in the early 1950s, fallout reached a peak in 1963 and then declined rapidly following the implementation of the test ban treaty. A number of scientists have proposed that the weapons test fallout peak could be used to mark the start of the Anthropocene. Various geological archives preserve the record of fallout, though with varying degrees of fidelity. They include polar snow and ice, marine and lacustrine sediments, and peat bogs. Bogs are ombrotrophic peatlands in that the plants growing there receive nutrients and contaminants exclusively from the atmosphere. The purpose of this study is to determine the fidelity of 241Am records in peat bog cores.
Specifically, we compare the position of the 241Am concentration peak with the 1963 depth determined by 210Pb dating. We use 39 peat cores from Europe, North America, and Indonesia collected by our team during the past 30 years for studies of atmospheric deposition of trace metals, all of which had been independently dated using 210Pb. We find that 18 of the cores provide an excellent agreement between the 241Am and 210Pb dates, 12 were in good agreement, and 9 agreed poorly. Possible reasons for the discrepancy in the 9 cores with the poor agreement are 1) the sensitivity of the gamma spectrometer for detecting 241Am, and 2) disruptions to the fallout records caused e.g. by disturbances to the peat bog or changes in the peat topography or hydrology. Small scale horizontal and vertical variations in bogs help explain why in a triplicate of peat cores collected from Wildseemoor in the Black Forest of Germany, excellent agreement was found in one core, good agreement in a second, and poor agreement in the third. A peat core collected from Gola di Lago, a small fen in Switzerland, showed excellent agreement; this suggests that samples from minerotrophic peatlands may also be useful to mark the start of the Anthropocene.

How to cite: Oleksandrenko, A., Appleby, P., Noernberg, T., and Shotyk, W.: Americium-241 in peat bogs as a marker of the beginning of the Anthropocene: examples from Europe and North America., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3744, https://doi.org/10.5194/egusphere-egu21-3744, 2021.

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