Changes in Cs-137 concentrations in river-bottom sediments and their factors in Fukushima Prefecture rivers

The Fukushima Daiichi Nuclear Power Plant accident (FDNPP) in 2011 resulted in the release of large amounts of Cs-137 into the atmosphere. Cs-137 deposited on land was mainly distributed in forests, but some of it has been discharged to the sea through rivers. The dissolved and suspended forms of Cs-137 in rivers have been focused on, and it is known that the discharge mechanism and concentration formation of Cs-137 differ depending on the land use in the river basin. On the other hand, there are few cases that focus on the dynamics of Cs-137 in river bottom sediments. River-bottom sediment is less likely to flow downstream than suspended sediments, so contamination in the downstream area may be long-term.
We will clarify the migration mechanism of Cs-137 in rivers including river-bottom sediment.Therefore, we will analyze data collected from 2011 to 2018 in 89 watersheds in Fukushima prefecture. In analyzing the data, we removed sampling points with brackish water using electrical conductivity and corrected for particle size to standardize the surface area of particles that absorb Cs-137.As a result, it was found that unlike dissolved and suspended forms, the Cs concentration in river-bottom sediments can increase within the initial year. This is related to the average initial deposition in the watershed and the amount of initial deposition at the river-bottom sediment sampling sites, with a tendency to increase with relatively higher initial deposition in the upstream area. It was also known that the decrease in suspended Cs concentration was more pronounced when anthropogenic activities in the watershed were more active, but there was no clear relationship between land use in the watershed and changes in river-bottom sediment Cs concentration. This indicates that suspended sediment Cs concentrations are controlled by initial deposition to suspended sediment production sources, whereas river-bottom Cs concentrations are controlled by multiple factors such as sediment traction and Cs supply from river water.