Dynamic change of dissolved Cs-137 from headwaters to downstream in the Kuchibuto River catchment

The Fukushima Daiichi Nuclear Power Plant (FDNPP) accident on March 11, 2011 resulted in the release of large amounts of radioactive cesium-137 (137Cs) into the environment. It is important to characterize the Cs-137 dynamics throughout the river from the headwaters to the downstream. Previous studies have suggested the importance of dissolved forms of Cs-137 in organic matter in small watersheds and dissolved forms in suspended solids in large watersheds. Since the concentration of suspended-form Cs has been shown to decrease significantly after decontamination in evacuated areas (Feng et al. 2022), this rapid decrease in suspended-form Cs-137 concentration can be used to determine the cause of dissolved-form Cs. Therefore, we attempted to evaluate whether the dissolved Cs-137 was derived from organic matter or suspended solids by comparing data before and after decontamination.

 The objective of this study is to compare the decreasing trends of Cs-137 concentrations in decontaminated and undecontaminated areas based on long-term monitoring of suspended solids, dissolved solids, and coarse organic matter Cs-137 concentrations since 2011. The study area includes four headwater basins and four river basins (eight sites in total) in the Kuchibuto River watershed in the Yamakiya district of Fukushima Prefecture, located approximately 35 km northwest of the FDNPP.

In the Kuchibuto River watershed, a large inflow of decontaminated soil with low Cs-137 concentrations due to an increase in the amount of bare land caused by decontamination resulted in a rapid decrease in the concentration of suspended-form 137Cs in the decontaminated area in the headwaters and in the upper reaches of the river. However, no clear effect of decontamination was observed in the concentrations of dissolved Cs-137 and Cs-137 in coarse organic matter. Comparison of the slopes of Cs-137 concentrations in the suspended, dissolved, and coarse organic matter showed that the slope of the dissolved form was similar to that of the coarse organic matter in the source watersheds, and similar to that of the SS in the downstream watersheds. These results suggest that the contribution of dissolved Cs-137 from organic matter in small watersheds and that from suspended solids in large watersheds is significant.