Gamma spectroscopy for geological studies

Gamma Ray spectroscopy is used in a large number of interdisciplinary applications, providing information on the identity of radioactive nuclides and allows their quantitative determination. 

Gamma Rays are electromagnetic radiations of nuclear origin and their detection is not a direct one, as it depends on the production of secondary particles which can be collected together to produce an electric signal.

Of all detector types, we prefer semiconductor ones, particularly Hyper-Pure Germanium detectors, which have very high efficiencies and excellent energy resolution. Following the sample type, occasionally the computerized analysis of the spectra has to be adapted or customized. The enormous differences between the environmental samples we need to face (from air filters to sediment, water to organic matter) drove us to develop protocols which have a general structure/pattern/methodology, but different approaches when it comes to treat the different matrices, would they be homogenous or not.

The opposite extremes in terms of use of Gamma Ray spectroscopy are the low and high count rate systems. Our job is to evaluate limits, to adapt to the statistical conditions, to calculate correction factors in order to get the results as close as possible to the reality.

Among our strengths there are various non standcard protocols, but also the use of information from the sum (coincident) peaks in order to acknowledge source activity and volume distribution; if the study is based only on the simple gamma peaks, the only information one would get is a large domain of possible positions of the source, without clear activity information. Another important topic is the information on the source homogeneity which is given by the count rates for peaks of different nature.

Our work is mainly experimental; most of the experiments are meant to be performed in the laboratory, as an interdisciplinary approach to nuclear and environmental science. One very important issue to consider in this field is the necessity to adapt to the changing radiation background, no matter the origins of the modifications. Also, the possibility of performing in situ gamma spectrometry is not to be neglected, as it offers multuple benefits, as on the spot analysis, quick tests, feasibility studies, accident dosimetry or simply mapping.

Additionally, we perform neutron activation on the samples, which means we can get the initially non-emitting nuclei to de-excite by gamma radiation: following neutron capture, the activated nuclei disintegrate by a beta process and subsequently emit characteristic gamma radiation, which helps un identify initially "silent" isotopes, bringing precious additional information.

 

Our results obtained experimentally and by Monte Carlo simulations in hypothesis testing of homogeneity properties and/or hot spots in volume sources are now being patented. Also, we seek to develop the quantum correlated gamma spectroscopy field, as it is emerging with new possibilities of treating entangled photons from environmental materials and specimens. Our main purpose for this event is to seek for partnership opportunities accross Europe.