EGU2020-11662
https://doi.org/10.5194/egusphere-egu2020-11662
EGU General Assembly 2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

Composition and Properties of the Natural Aerosol over the Boreal and Tropical Forests

Hans-Christen Hansson1, Paulo Artaxo2, Meinrat Andreae3, and Markku Kulmala4
Hans-Christen Hansson et al.
  • 1Department of Environmental Science, Stockholm University, Stockholm, Sweden
  • 2Institute of Physics, University of Sao Paulo, Sao Paulo, Brazil
  • 3Max Planck Institute for Chemistry, Mainz, Germany
  • 4Institute for Atmospheric and Earth System Research INAR, University of Helsinki, Finland

We, together with 50 of our colleagues present a review on the interaction between tropical and boreal forests and the atmosphere, especially addressing their influence in the climate system. With its emissions of VOCs, aerosols and trace gases, with strong atmosphere interactions, forests are a key component of the climate system. These emissions and atmospheric processing regulates atmospheric chemistry and are the major source of cloud condensation nuclei (CCN) affecting cloud formation and development, and thus temperature and precipitation. Emissions from forests are thus closely connected to the hydrological and the carbon cycles, being  an essential integrated part of the climate system.

In terms of meteorology, tropical and boreal forests are very different. Temperature, solar radiation, precipitation, evapotranspiration, albedo, cloud structure and cover, convection etc., are all very different. However, the aerosols in the two systems show similarities as Primary Biological Aerosol Particles are the major component (70%) of coarse mode particles in Amazonia while Secondary Organic Aerosol in the tropics are mainly isoprene driven giving a slightly more hygroscopic SOA than the boreal monoterpene driven SOA. The organics constitutes 70 to 85% of PM1 mass for both boreal and tropical forests. In Amazonia, sulfates, nitrates and BC shows very low concentrations, while the boreal sites shows 2-3 times higher concentrations. The Siberian continental site and Amazonian site show remarkable similarities in the lack of new particle formation (NPF) which will be  discussed.

In the tropics dry season and boreal spring and early summer, increasing biomass burning emissions in both forest types dominates the aerosol composition, with high OC and BC concentrations while anthropogenic pollution influences boreal forest atmospheric composition during wintertime. The changes in diffuse to direct radiation due to scattering aerosols has important effects in tropical forests but minor in boreal, enhancing the net ecosystem exchange by 30% and 10% respectively. Thus the natural forest emissions affects the direct as well as the indirect forcing.

An Amazonia high altitude NPF process chain was recently observed at the top of the troposphere, and is an interesting interaction between forest emissions, cloud transport and processing and particle formation and aging at high altitudes that are brought back to the boundary layer, populating the CCN. For boreal forests, the complex relationship between GPP, BVOC, SOA, CCN, clouds, radiation, temperature and CO2 show multiple pathways and feedbacks, and some of them can be quantified. All showing the complexity of the interaction between forests, atmosphere and climate.

How to cite: Hansson, H.-C., Artaxo, P., Andreae, M., and Kulmala, M.: Composition and Properties of the Natural Aerosol over the Boreal and Tropical Forests, EGU General Assembly 2020, Online, 4–8 May 2020, EGU2020-11662, https://doi.org/10.5194/egusphere-egu2020-11662, 2020

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Presentation version 1 – uploaded on 01 May 2020
  • CC1: Comment on EGU2020-11662, Santiago Gassó, 04 May 2020

    Hello

    I wonder have you carried out any analysis to determine the enantiomer state of the different terpenes and other organics known to have isomers?

     

    Santiago

    • AC1: Reply to CC1, Hans-Christen Hansson, 04 May 2020

      This is a review, about 105 pages long, so we present few new  data. It is mainly a review and syntheses of existing litterature. There is a comprehensive presentation of BVOC emissions and subsequent chemical processes giving observed gaseous and condensed organic component. Monoterpenes and sesquiterpenes are discussed in detail. Professor Alex Guenther, uUniversity of California, Irvine is the key author of the BVOC part. The paper is submitted and will probably be in press in a few months.