Zero-shot learning of aerosol optical properties with graph neural networks

Black carbon (BC), a strongly absorbing aerosol sourced from combustion, is an important short-lived climate forcer. BC’s complex morphology contributes to uncertainty in its direct climate radiative effects, as current methods to accurately calculate the optical properties of these aerosols are too computationally expensive to be used online in models or for observational retrievals. Here we demonstrate that a Graph Neural Network (GNN) trained to predict the optical properties of numerically-generated BC fractal aggregates can accurately generalize to arbitrarily shaped particles, including much larger (10x) aggregates than in the training dataset. This zero-shot learning approach could be used to estimate single particle optical properties of realistically-shaped aerosol and cloud particles for inclusion in radiative transfer codes for atmospheric models and remote sensing inversions. In addition, GNN’s can be used to gain physical intuition on the relationship between small-scale interactions (here of the spheres’ positions and interactions) and large-scale properties (here of the radiative properties of aerosols).