Aerosol-cloud interactions under fine-mode and coarse-mode aerosol conditions over the monsoon region of Pakistan

Abstract

The densely populated monsoon region of Pakistan, influenced by a diverse mix of natural and anthropogenic aerosols, provides a natural laboratory to investigate aerosol impacts on cloud properties. Using a decade-long (2015–2024) dataset from MODIS, MERRA-2, and ERA5, we examine the response of non-precipitating warm clouds to fine-mode and coarse-mode aerosols. We find positive correlations between aerosol optical depth (AOD) and cloud effective radius (CER), with stronger sensitivity to fine-mode AOD. The relationships of AOD with cloud optical thickness (COT) and liquid water path (LWP) are generally negative, but more pronounced for coarse-mode AOD. These aerosol-cloud relationships are strongly modulated by meteorological conditions: low relative humidity and low lower-tropospheric stability enhance the negative AOD–COT and AOD–LWP responses. Additionally, the sensitivity of aerosol-cloud relationships to meteorology is greater for fine-mode AOD than coarse-mode. These results highlight the importance of aerosol size and ambient meteorology in determining cloud microphysical responses, providing insight into aerosol cloud interactions in a region critical for South Asian climate.